Background: Lung cancer is the leading cause of cancer-related death worldwide [1] and presents a significant clinical challenge due to chemoresistance. First-line treatment of lung cancer includes the use of platinum-based chemotherapy drugs (cisplatin, carboplatin). These drugs function by cross-linking DNA to impede cell proliferation, while also inducing the generation of reactive oxygen species (ROS) intracellularly. SLC7A11 has been identified as a pivotal gene involved in tumour metabolism and is highly expressed in cancer cells [2,3]. SLC7A11 is a key regulator of amino acid metabolism and is highly expressed in cancer cells. SLC7A11 protects cells from chemotherapy-induced ROS by promoting glutathione synthesis to stabilize ROS. Sulfasalazine (SSZ), a pharmacological inhibitor of SLC7A11, is already used in clinical settings to treat arthritis. We propose that the inhibition of SLC7A11 function with SSZ or gene-altering small-interfering RNA (siRNA) could enhance the effectiveness of platinum-based chemotherapy in lung cancer cells.
Aims: To determine the effectiveness of SSZ or SLC7A11-siRNA in combination with platinum chemotherapy to inhibit lung cancer cell growth.
Methods: SLC7A11 protein expression was measured using western blotting in human lung cancer cells (A549, H1299, H441, H1975). Lung cancer cell growth in the absence or presence of SSZ (0.5-2mM), cisplatin (1.5-6uM), carboplatin (10-20uM) or oxaliplatin (1-4uM) was examined using trypan blue staining and clonogenic assays. Apoptosis and ROS was measured using Annexin V and CellROX staining and flow cytometry. Glutathione levels were measured using an enzyme assay. SLC7A11-siRNA was delivered to lung cancer cells using Lipofectamine2000®, and cell viability and drug sensitivity assessed by trypan blue staining and Alamar blue drug assays.
Results: Lung cancer cells express SLC7A11. In A549 and H1299 cells, SSZ significantly decreased cell viability and proliferation when used in combination with cisplatin, carboplatin and oxaliplatin (*p≤0.05) compared to drugs alone. Mechanistically, we confirmed a significant depletion of glutathione and its active enzyme facilitator, glutathione peroxidase 4 (GPX4) after SSZ treatment within 24h (*p<0.05) and an increase in apoptosis when used in combination with platinum chemotherapy (**p≤0.01). SLC7A11-siRNA also decreased cell viability (*p<0.05) and sensitised A549 cells to cisplatin treatment (*p≤0.05).
Conclusions/Translational significance: These findings suggest that SLC7A11 is a promising therapeutic gene target to increase the chemosensitivity of platinum-based chemotherapy drugs in lung cancer cells. The addition of SSZ to platinum-based therapies for lung cancer may improve drug efficacy in the clinic to ultimately improve patient survival. It may also lower chemotherapy concentrations required for effective treatment.